Materials Science and Engineering
Laboratory name
Quantum Interface Laboratory   
Laboratory title
量子構造の表面・界面の光・電子・化学物性の基礎研究・制御・応用
Laboratory overview
量子ナノ構造を物理的・化学的に作製し、その表面・ 界面における電子的な挙動の某礎研究を行っている。応用として、光・ 電子・化学的な機能の制御と新たな機能創出を目指している。 特に電子物理と化学の境界領域に焦点を当てた研究に取り組んでいる。
Main research themes
・量子構造表面界面の光・電子物性
・III-V族半導体のエピタキシャル結晶成長機構
・ナノ粒子のコロイダル合成と物性
・量子構造によるエネルギー変換素子
Individual research theme
  • Passivation-capping of III-V semiconductor quantum structures by oxides

    神谷 格, Ronel Christian Intal ROCA, 岩田 直高

    2017

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    Outcome:

    2024
    The mechanisms of passivation by metal oxide capping has been investigated. It has been suggested that organometallic precursors change the state of the oxide at the surface upon reaction.

    2023
    By comparing passivation capping by ZnO and AlOx, it was found that the crytallinity of the formed film and the self-cleaning process of the precursors play an important role in determining the properties of the surface quantum dots.

    2022
    By passivating surface InAs quantum dots, enhanced PL intensity with reduced wavelength peak was obtained.

  • Development of InGaAs-based quantum structures by SML growth

    神谷 格, Ronel Christian Intal ROCA

    2017

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    MBE growth of InGaAs quantum structures using submonolayer (SML) stacking is studied thereby precisely controlling the structure and electronic properties of the quantum structures.
    Further, the potential of applying such structures to spintronics is investigated.

    Outcome:

    2024
    Studies on the dependence of parameters such as As pressure, growth interrupt, or InAs deposition, on the formation of nanostructures formed by submonolayer (SML) stack growth.

    2023
    Control of spin was shown by illuminating these 2D and 3D structures by circular polarized excitation light.

    2022
    The transition of 2D-3D in submonolayer growth has been studied and the critical conditions were identified and the mechanisms were studied.

  • Photon upconversion using InAs quantum structures

    神谷 格, Ronel Christian Intal ROCA

    2017

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    Outcome:

    2024
    Modified preparation of quantum discs by SML stacking and measurement of their optical properties.

    2023
    Shown that quantum discs can be prepared by using SML stacking.

    2022
    Preparation of quantum discs that are considered to be a strong candidate for photon upconversion is being investigated.

  • Fundamental studies of semiconductor interfaces

    神谷 格, Ronel Christian Intal ROCA

    2017

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    Outcome:

    2023
    By comparing different precursor materials, the basic guidelines for passivating InAs surface quantum dots were proposed.

    2022
    The recipes and the mechanisms of passivating InAs surface quantum dots were studied.

  • Epitaxial crystal growth and its mechanisms

    神谷 格, Ronel Christian Intal ROCA

    2017

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    Outcome:

    2024
    2D and 3D quantum structures have been grown usingU controlled SML stack growth, and their electronic properties have been studied by spin-polarized PL.
    Basic studies on the mechanisms of SML stack growth has also been investigated.

    2023
    Controlled growth of 2D and 3D quantum structures by SML stack growth has been successfully demonstrated, and its device applications are under investigation.

    2022
    The transition of 2D-3D in submonolayer (SML) stack growth has been studied and the critical conditions were identified and the mechanisms were studied.

  • Preparation of functional thin films and their properties

    神谷 格

    2017

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    Outcome:

    2023
    Strain-free passivation capping of surface quantum dots by ALD metal oxide thin films was successfully demonstrated, and its device applications are under investigation.

    2022
    Atomic layer deposition (ALD) of metal oxide thin films are being investigated.

  • Exploration of oxide light emitter

    神谷 格, 岩田 直高

    2020

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    An attempt to realize short wavelength emission from oxide thin films.

    Outcome:

    2024
    Exploration of methods for improving the films.

    2023
    Organizing the lab/equipment for improving the films.

    2022
    Short wavelength light emission from oxide films indicated.

  • Towards deterministic fabrication of QD single-photon sources for quantum information applications

    Ronel Christian Intal ROCA

    2025 - 2027

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    To purpose is to investigate the deterministic fabrication of single-photon sources based on epitaxial quantum dots.

  • 2D to 3D growth transition of Submonolayer InAs/GaAs nanostructures

    Ronel Christian Intal ROCA

    2020

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    Submonolayer (SML) deposition by MBE is a method that was proposed to assembled InAs nanostructure while maintaining 2D (layer-by-layer) growth. However, it has recently been shown that under certain growth conditions, a transition from 2D to 3D growth regime occurs during SML growth. This process is interesting for both fundamental physics and potential applications.

    Outcome:

    2024
    Further study of the 2D-3D transition during InAs/GaAs submonolayer deposition has been carried out. We have recently demonstrated fine control of the 3D QD density down to low densities of less than 1QD per square micron, which is beneficial for quantum information applications. Some of our latest results have been presented at the SPIE PW 2025 conference.

    2023
    We were able to investigate various factors that affect the 2D to 3D transition during SML growth. Some of the results have been presented in the JSAP Autumn Meeting 2023.